Add time:07/26/2019 Source:sciencedirect.com
A personal note in celebration of Professor Herrmann's 70th birthday, the author describes how the successful preparation of H3C99TcO3 and the still unsolved task of preparing [Cp*99TcO3] powered ultimately a plethora of organometallic 99Tc chemistry. Driven by the need for Technetium (cas 109581-73-9) carbonyl complexes, the red wire leads from [99TcCl3(CO)3]2- over the related [99mTc(OH2)3(CO)3]+ and [(L3)99TcO3]+ finally to [99Tc(arene)2]+ complexes. It is shown how, from the fundamental search for [Cp*99TcO3], useful molecules for application in molecular imaging emerged.
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