Add time:08/15/2019         Source:sciencedirect.com

A new three-dimensional diamagnetic metal nitronyl nitroxide radical coordination polymer with an aqua cadmium cyanide framework Cd(NIT4py)(H2O)Cd(CN)4·H2O 1, was synthesized. X-ray crystallography reveals that the structure consists of 3D aqua cadmium cyanide built up by octahedral CdII coordinating to NIT4py and tetrahedral CdII (CN)4 units. Magnetic measurements show that the χmT values are nearly constant at higher temperature. The lower χmT values at lower temperature are related to intermolecular antiferromagnetic interactions of the radicals, which arise due to the hydrogen bonded network (TN = 21 K).

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