Add time:07/16/2019         Source:sciencedirect.com

In this communication, we account the synthesis, spectroscopic, crystal structure, and photophysical and DFT studies of N-phenylthiazole-5-carboxamide derivatives. Synthesis of N-arylthiazole-5-carboxamideswas obtained using eco-friendly conditions. Two compounds were synthesized with high yield under eco-friendly conditions. The conformed spectral data were reliable with the chemical structures of 2-bromo-4-methyl-N-arylthiazole-5-carboxamides. The single crystal study additionally endorses its three-dimensional structure, molecular shape, hydrogen bonding and the nature of short contacts. The crystal structure reveals that arylthiazole-5-carboxamides retains a non-planar structure with two crystals have shifted packing within the crystal unit. Its computed photophysical properties also in good agreement with the experimental findings. Moreover, UV–visible and fluorescence spectral studies evidence that the compound exposes proper absorption and fluorescence properties.

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