Add time:08/21/2019         Source:sciencedirect.com

The reactions of the phenyl radical (C6H5) with 1-Butyne (cas 107-00-6) (HCCC2H5) and 2-butyne (CH3CCCH3) were studied in a crossed molecular beam machine to shed light on the formation of C10H10 isomers in combustion flames. Combining these data with electronic structure calculations, we find that both reactions involve indirect scattering dynamics and are initiated by additions of the phenyl radical with its radical center to the acetylenic carbon atoms. The reaction intermediates fragmented through the ejection of hydrogen atoms yielding 1-phenyl-3-methylallene and 1-phenyl-1-butyne (both from 1-butyne) as well as 1-phenyl-1-methylallene (from 2-butyne).

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