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B
hydroperoxyl radical
Conditions | Yield |
---|---|
With perchloric acid; oxygen In acetonitrile Kinetics; | A 100% B n/a |
carbon disulfide
dihydrogen peroxide
oxygen
A
sulfur dioxide
B
hydroperoxyl radical
Conditions | Yield |
---|---|
In gas Kinetics; byproducts: HS; other Radiation; H2O2 is photolysed at 266 nm (Nd:YAG laser) in a flow reactor, addn. of CS2 (NO) and O2 (N2); HO2 yield measurement by LMR (laser magnetic resonance), SO2 yield measurement by CIMS (chemical ionization mass spectometry); | A 90% B 95% |
Conditions | Yield |
---|---|
With synthetic air; oxygen In gaseous matrix Kinetics; C2H4, CO and synthetic air mixture addn. into O3/O2 flow; | 66% |
Conditions | Yield |
---|---|
With synthetic air; oxygen In gaseous matrix Kinetics; byproducts: hydroxyethylperoxy radical; C2H4 (1-3 ml/min) and synthetic air (3 ml/min) mixture addn. into O3/O2 flow; | A 20% B 39% |
hydroxyl
chlorine monoxide
A
hydrogenchloride
C
oxygen
D
hydroperoxyl radical
Conditions | Yield |
---|---|
In gas Kinetics; between 218 and 298 K, OH source: F + H2O or H + NO2, ClO source: Cl + O3, reaction carried out in a discharge-flow system; | A 9% B n/a C n/a D n/a |
In gaseous matrix Kinetics; carrier gas: He; hydroxyl radicals were prepared by the reaction between H and NO2; ClO radicals were prepared by the reaction between O3 an Cl; resonance-fluorescence measurements; |
Conditions | Yield |
---|---|
In neat (no solvent) Kinetics; byproducts: C2H4, C2H5O2; Irradiation (UV/VIS); reaction of O2 with C2H5 radicals formed by flash-light photolysis (22 °C, 5-100 Torr total pressure); 99.9% of C2H5 reacted with formation of C2H5O2; rate constant;; | 0.1% |
In neat (no solvent) Kinetics; byproducts: C2H4; reaction of C2H5 radicals with O2 at T<320 °C; mechanism;; |
Conditions | Yield |
---|---|
In gas Kinetics; CH4-O2 reaction at 1100 °C and total pressure of 10 Torr; HO2 decay (1. order);; mass spectroscopy;; | |
In neat (no solvent) CH4-O2 flames (12 Torr);; mass spectroscopy; assignment to HO2 is doubtful;; | |
In neat (no solvent) CH4-O2 flames (70 Torr);; mass spectroscopy;; | |
In neat (no solvent) byproducts: CH3, H2O2; reaction of 5 Torr CH4 with 3 Torr O2 at 1090 °C (reaction period 10E-2 s); collision yield; following reaction;; mass spectroscopy;; | 0.05% |
In neat (no solvent) examination of the CH4-O2 reaction;; |
Conditions | Yield |
---|---|
Kinetics; byproducts: OH, H2O, O2; at 298-386 K and 15-150 Torr; | |
In neat (no solvent) Kinetics; byproducts: OH, H2O, O2; gaseous H2O2 was mixed with O+O2; rate constant;; | |
In neat (no solvent) |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; reaction of OH (produced on reaction of H + NO2 -> OH + NO) and O3 (He carrier gas, 1.5 - 4 Torr, 300 K - 423 K); |
Conditions | Yield |
---|---|
With water; acetic acid In water Kinetics; byproducts: O2; Irradiation (UV/VIS); | |
In neat (no solvent) Kinetics; byproducts: O2; OH radicals formed from H+NO2 reacted with O3; rate constant;; UV absorption measurements;; |
Conditions | Yield |
---|---|
With nitrogen In gas Kinetics; kinetic of react. of OH radical with H2O2 studied over temp. range 96-296 K; H2O2/N2 gas expanded through Laval nozzle; laser-induced fluorescence of OH radical used as probe; | |
In gas Kinetics; kinetics studied at 250-1250 K by means of UV spectroscopy; | |
In gaseous matrix Kinetics; 245-423 K; total pressure=45-500 torr; in He stream, in contact with quarz, Pyrex or Teflon only; not sepd.; |
Conditions | Yield |
---|---|
In gas fast-flow discharge system (according to: T. E. Kleindienst, B. J. Finlayson-Pitts, J. Chem. Phys. Lett. 61 (1979) 300), halocarbon wax or boric acid coated flow tube, H or O3 excess; resonance fluorescence technique, titration of H; |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; other Radiation; laser photolysis (mixt. of O3 with He (1:1E+4), KrF excimer laser); detection by time-resolved atomic absorption spectroscopy; | |
fast-flow discharge system (room temp., excess of O3, bychoise addn. ofCO or NO); |
dihydrogen peroxide
ozone
A
hydroxyl
B
oxygen
C
hydroperoxyl radical
Conditions | Yield |
---|---|
In water Kinetics; |
water
A
hydroxyl
B
hydrogen
C
dihydrogen peroxide
D
hydroperoxyl radical
Conditions | Yield |
---|---|
Kinetics; other Radiation; effect of radiation type and scavanger concn. in water radiolysis; |
hydrogen sulfide
water
oxygen
A
sulfur dioxide hydrate
B
SO3 * water
C
sulfuric acid
D
sulfur dioxide
E
hydroperoxyl radical
Conditions | Yield |
---|---|
In solid matrix Irradiation (UV/VIS); further products; 270-420 nm photolysis in O2-matrix at 13 K (4-14 h); product ratio depending on matrix composition; not isolated, detected by IR; |
water
oxygen
A
hydrogen peroxide water
B
dihydrogen peroxide
C
ozone
D
hydroperoxyl radical
Conditions | Yield |
---|---|
In solid matrix Irradiation (UV/VIS); photolysis at 13 K for 1.8 h (λ > 220 nm); not isolated, detected by IR; |
hydrogen cyanide
A
isocyanic acid
C
carbon nitride
D
hydroperoxyl radical
Conditions | Yield |
---|---|
Ar/HCN is codeposited with O atoms (produced by microwave discharge of Ar/O2)on cold CsI window; IR matrix isolation study; |
silver (I) ion
hydroperoxide anion
A
silver
B
hydroperoxyl radical
Conditions | Yield |
---|---|
In water mechanism of H2O2-decomposition discussed;; | |
In water mechanism of H2O2-decomposition discussed;; |
dihydrogen peroxide
carbonate radical anion
A
hydrogen carbonate
B
hydroperoxyl radical
Conditions | Yield |
---|---|
In water pH=6.3, 24°C; |
Conditions | Yield |
---|---|
In gaseous matrix byproducts: HCl; He carrier gas; |
Conditions | Yield |
---|---|
With oxygen In gas Kinetics; Flash photolysis-shock tube react.of O2/Ar-mixt. with H (produced by photodissociation of NH3 or H2O).; Rate consts. between 746 and 1705 K at various pressures given.; |
Conditions | Yield |
---|---|
In gas Kinetics; under Ar, mixed, reacted at 293 K (P=1 kPa); ESR, gas chromy.; |
Conditions | Yield |
---|---|
In gas Kinetics; rate coefficients measured via OH absorption behind reflected shock waves at 950-3100 K; H2/O2/Ar mixtures prepared manometrically and allowed to stand for at least 48 h; |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; H and O2 reacted in excess of Ar in fast flow-discharge tube at 2-10 Torr and at 231-512 K; detected by mass spectrometry and GC chromy; | |
With He or N2 or H2O In gas Kinetics; other Radiation; reacting H atoms with O2 in the presence of He, N2 or H2O (microwave discharge, pressure 0.25 - 1 Torr); | |
With nitrogen In gas Kinetics; |
Conditions | Yield |
---|---|
Kinetics; in O2/H2 flame; fluorescence spectroscopy; |
Conditions | Yield |
---|---|
With isopropyl alcohol; 12-tungstoferric acid In water Kinetics; Irradiation (UV/VIS); soln. contg. heteropolytungstate ion (2E-6 M) and i-PrOH (1.7 M) subjected to 10E-6 s photoflash in presence of O2 (2E-4 M) at pH 1.0 (0.05 M H2SO4); | |
With isopropyl alcohol; sodium phosphotungstate In water Kinetics; Irradiation (UV/VIS); soln. contg. heteropolytungstate ion (2E-6 M) and i-PrOH (1.7 M) subjected to 10E-6 s photoflash in presence of O2 (2E-4 M) at pH 1.0 (0.05 M H2SO4); | |
With isopropyl alcohol; sodium metatungstate In water Kinetics; Irradiation (UV/VIS); soln. contg. polytungstate ion (2E-6 M) and i-PrOH (1.7 M) subjected to10E-6 s photoflash in presence of O2 (2E-4 M) at pH 1.0 (0.05 M H2SO4); | |
With isopropyl alcohol; 12-tungstosilicic acid, K-salt In water Kinetics; Irradiation (UV/VIS); soln. contg. heteropolytungstate ion (2E-6 M) and i-PrOH (1.7 M) subjected to 10E-6 s photoflash in presence of O2 (2E-4 M) at pH 1.0 (0.05 M H2SO4); |
formyl radical
oxygen
A
carbon monoxide
B
hydroperoxyl radical
hydrogen sulfide
oxygen
A
sulfuric acid
B
sulfur dioxide
C
sulfur trioxide
D
ozone
E
hydroperoxyl radical
Conditions | Yield |
---|---|
byproducts: H2O*SO2, H2O*SO3; Irradiation (UV/VIS); in solid O2, 15K; H2O*SO2 and H2O*SO3 present in significant amounts; detected by IR; |
hydrogen sulfide
oxygen
A
sulfur dioxide hydrate
B
SO3 * water
C
sulfuric acid
D
sulfur dioxide
E
hydroperoxyl radical
Conditions | Yield |
---|---|
In solid matrix Irradiation (UV/VIS); further products; 270-420 nm photolysis in O2-matrix at 13 K (4-14 h); product ratio depending on matrix:solute ratio (200-8000); not isolated, detected by IR; |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; Cl concn. 3E11 - 3E12 molecule/cm3, HO2 concn. 1E10 - 5E11 molecule/cm3,236 K, 1 Torr of He; | A 94.5% B n/a |
In gaseous matrix Kinetics; Cl concn. 3E11 - 3E12 molecule/cm3, HO2 concn. 1E10 - 5E11 molecule/cm3,256 K, 1 Torr of He; | A 79.4% B n/a |
In gaseous matrix Kinetics; Cl concn. 3E11 - 3E12 molecule/cm3, HO2 concn. 1E10 - 5E11 molecule/cm3,276 K, 1 Torr of He; | A 74.8% B n/a |
In gaseous matrix Kinetics; Cl concn. 3E11 - 3E12 molecule/cm3, HO2 concn. 1E10 - 5E11 molecule/cm3,296 K, 1 Torr of He; | A 70.4% B n/a |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; Cl concn. 2E10 - 5E10 molecule/cm3, HO2 concn. 4E11 - 4E12 molecule/cm3,336 K, 1 Torr of He; | A 26% B n/a |
In gaseous matrix Kinetics; Cl concn. 2E10 - 5E10 molecule/cm3, HO2 concn. 4E11 - 4E12 molecule/cm3,316 K, 1 Torr of He; | A 23.6% B n/a |
In gaseous matrix Kinetics; Cl concn. 2E10 - 5E10 molecule/cm3, HO2 concn. 4E11 - 4E12 molecule/cm3,296 K, 1 Torr of He; | A 18.6% B n/a |
Conditions | Yield |
---|---|
Kinetics; byproducts: O2; rate constant;; | |
In sulfuric acid Kinetics; byproducts: O2; other Radiation; decrease of HO2 which was formed by pulsed or continuous electron radiation of H2O2-O2-H2SO4 soln.; rate constant;; | |
In gaseous matrix Kinetics; byproducts: O2; 298 K, He or Ar present at total pressures 75 - 730 torr; |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; reaction of O2H (produced on reaction of H + O2 + M -> HO2 + M) and O3 (He carrier gas, 1.5 - 4 Torr, 245 K - 365 K); | |
In gas Kinetics; discharge-flow system at room temp.;; | |
In gas Kinetics; rate constant determined in the temp. range 233-400 K; |
Conditions | Yield |
---|---|
byproducts: OH; |
Conditions | Yield |
---|---|
In water |
Conditions | Yield |
---|---|
Kinetics; in O2/H2 flame; fluorescence spectroscopy; |
Conditions | Yield |
---|---|
Kinetics; in O2/H2 flame; fluorescence spectroscopy; |
Conditions | Yield |
---|---|
Kinetics; in O2/H2 flame; fluorescence spectroscopy; |
Conditions | Yield |
---|---|
In gaseous matrix Kinetics; byproducts: O2; react. of atomic oxygen and HO2 radicals at 2 Torr, 299 K in a He flow; not isolated, detected by resonance fluorescence technique; | |
In gaseous matrix Kinetics; byproducts: O2; educts were produced by laser pulsed photolysis of O3 and H2O2 in N2 or Ar at 10-500 Torr; detection by time-resolved fluorescence; | |
In neat (no solvent) Kinetics; byproducts: O2; rate constant;; |
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